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I see a very well documented way, if a user is not enabled to decrypt the boot volume, to enable that user: just go into the FileVault control panel, and if there are users not permitted to boot the system, there will be a message so-indicating, and a button that will bring up a dialog for enabling them.

I have the converse problem: I have a user FileVault-enabled user, who should NOT be.

Is there a way to do this?

bmike
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This is indeed a duplicate of Disable a user's ability to unlock a FileVault 2 volume at startup/login time, i.e., sudo fdesetup remove -user username

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    Excellent! Well close this and your words will help others search and know the questions are solved with the same answer. +1 – bmike May 22 '23 at 19:20