I don't think it is possible at any altitude because the ISS has the wrong moment of inertia (mass distribution) for this.
Moments of inertia
As far as I understand it, to use gravity-gradient stabilization efficiently, you need to have the largest moment of inertia in the direction of the gradient; the zenith-nadir or vertical direction. You also need a source of damping force to remove energy in the oscillations that can build up over time due to any other torques. See for example this answer. See also this answer and the extensive series of comments be low it.
From Gravity Gradient Stabilization of Earth Satellites by R. E. Fischell as discussed in this answer (click for full size):

In the case of a long thin rod, there is a cancellation of terms and angular acceleration is independent of spacecraft length or mass. From this answer:
For some math, see (Help with my tensor tension; how to derive and calculate this rigid body gravity gradient torque?) and especially @Litho's answer. For a thin rod of mass $m$ and length $l$ in circular orbit, with a perpendicular moment of inertia $\frac{1}{12}ml^2$, rotating in-plane around the short axis, the torque (to first order) is given by
$$L_G = -\frac{GM_Eml^2}{8R_C^3}\sin 2\theta,$$
and the instantaneous angular acceleration is simply
$$\ddot{\theta} = -\frac{3GM_E}{2R_C^3}\sin 2\theta.$$
That's a pretty amazing result! With $GM_E$ of about 3.986E+14 m^3/s^2 and an altitude of 400 km, $\ddot{\theta}$ can be as large as 0.4 degrees per minute^2 at 45 degrees, and that is independent of length!
Aerodynamic drag
Let's compare that to an order of magnitude estimate of the angular acceleration due to aerodynamic drag on the ISS' solar panels.
The moment of inertia of ISS can be approximated with $\frac{1}{12}ml^2$ using a mass of about 400,000 kg and a length of about 70 meters I get a moment of inertia of about 1.6E+08 kg m^2.
I estimate a solar panel area of all the panels on one end of the ISS to be about 800 square meters. Using a simple model for drag force
$$F_D = \frac{1}{2} \rho v^2 C_D A$$
and high solar activity density at 400 km of about 5E-11 kg/m^3 and a worst case configuration, I get a drag force of about 1.2 Newtons at about 30 meters from the ISS' center of mass.
Using $\ddot{\theta} = 1.2 N \times 30 m / 1.6 \times 10^8 kg \ m^2$ I get an angular acceleration due to an unfortunate drag scenario of only about 0.05 degrees per minute squared, way below the torque that can be generated by the gravity gradient once the ISS starts tilting towards vertical orientation.
Conclusion
The ISS can't use gravity gradient stabilization to keep it in it's current orientation - long direction pointed forward. However it could certainly be used if you wanted to orient it nose-down. In that case the stabilization is much larger than even an unfortunate drag scenario, and it's probable that by articulating the solar panels properly you can use drag as the damping force to maintain stabilization.
From here:

Furthermore, if considering higher altitudes, tidal locking works by deformation of the body due to tidal force, it is quite possible that this effect would be negligible for a body as small as the ISS.
– M'vy Jun 05 '19 at 08:42